It would definately have to be the 音楽 from "Sweeney Todd: The Demon Barber of Fleet Street". I also 愛 the 音楽 to "Edward Scissorhands" and "The Nightmare Before Christmas"; pretty much anything によって Danny Elfman (he composes like EVERY Tim バートン movie soundtrack).
Oooooooooooh! Hairspray... Wait, no, Bridge to Terrabithia.... No, Twilight! Wait, wait! New Moon! No.... Eclipse!!! IDK, those are like, my most fave, not in order, but... I LIVE for movie soundtracks, haha. :)
There are lots of them...I like soundtracks from Pearl Harbor, Armageddon, Once Upon A Time In America(probably the best soundtracks ever), メリダとおそろしの森 Heart, Gladiator, Pirates Of The Caribbean and many many others.