White Destiny from Pretear. Morning Grace from Princess Tutu and Aiyaa Four Thousand Years were my two 上, ページのトップへ candidates, but since they're taken, I'll go with my current お気に入り song. I mean, just listen to it! This song is the reason I adore Yoko Ishida(she sings it, btw)!<3333 Pretear is the only アニメ I've ever watched where I didn't start skipping the intro after the first few episodes.
Another アニメ song I really 愛 is Brothers from FullMetal Alchemist. Vic Mignogna's English version is just so gorgeous, I can't even begin to explain it! It's even sadder if you've seen the アニメ and あなた know what Ed's been through... T~T
Brothers:
link White Destiny: